Catalytic Ammonia Reforming: Alternative Routes to Net-Zero-Carbon Hydrogen and Fuel

Luis Caballero, Nicholas Thornburg, Michael Nigra

Research output: Contribution to journalArticlepeer-review

7 Scopus Citations

Abstract

Ammonia is an energy-dense liquid hydrogen carrier and fuel whose accessible dissociation chemistries offer promising alternatives to hydrogen electrolysis, compression and dispensing at scale. Catalytic ammonia reforming has thus emerged as an area of renewed focus within the ammonia and hydrogen energy research & development communities. However, a majority of studies emphasize the discovery of new catalytic materials and their evaluation under idealized laboratory conditions. This Perspective highlights recent advances in ammonia reforming catalysts and their demonstrations in realistic application scenarios. Key knowledge gaps and technical needs for real reformer devices are emphasized and presented alongside enabling catalyst and reaction engineering fundamentals to spur future investigations into catalytic ammonia reforming.

Original languageAmerican English
Pages (from-to)12945-12956
Number of pages12
JournalChemical Science
Volume13
Issue number44
DOIs
StatePublished - 2022

Bibliographical note

Publisher Copyright:
© 2022 The Royal Society of Chemistry.

NREL Publication Number

  • NREL/JA-5400-81574

Keywords

  • ammonia energy
  • autothermal
  • hydrogen carrier
  • monolith
  • NOx emissions
  • reaction engineering
  • reforming catalysis
  • renewable fuel

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