TY - JOUR
T1 - Integrated Evaluation of Cost, Emissions, and Resource Potential for Algal Biofuels at the National Scale
AU - Davis, Ryan
AU - Kinchin, Christopher
AU - Fishman, Daniel
AU - Frank, Edward
AU - Johnson, Michael
AU - Jones, Susanne
AU - Skaggs, Richard
AU - Venteris, Erik
AU - Wigmosta, Mark
PY - 2014/5/20
Y1 - 2014/5/20
N2 - Costs, emissions, and resource availability were modeled for the production of 5 billion gallons yr-1 (5 BGY) of renewable diesel in the United States from Chlorella biomass by hydrothermal liquefaction (HTL). The HTL model utilized data from a continuous 1-L reactor including catalytic hydrothermal gasification of the aqueous phase, and catalytic hydrotreatment of the HTL oil. A biophysical algae growth model coupled with weather and pond simulations predicted biomass productivity from experimental growth parameters, allowing site-by-site and temporal prediction of biomass production. The 5 BGY scale required geographically and climatically distributed sites. Even though screening down to 5 BGY significantly reduced spatial and temporal variability, site-to-site, season-to-season, and interannual variations in productivity affected economic and environmental performance. Performance metrics based on annual average or peak productivity were inadequate; temporally and spatially explicit computations allowed more rigorous analysis of these dynamic systems. For example, 3-season operation with a winter shutdown was favored to avoid high greenhouse gas emissions, but economic performance was harmed by underutilized equipment during slow-growth periods. Thus, analysis of algal biofuel pathways must combine spatiotemporal resource assessment, economic analysis, and environmental analysis integrated over many sites when assessing national scale performance.
AB - Costs, emissions, and resource availability were modeled for the production of 5 billion gallons yr-1 (5 BGY) of renewable diesel in the United States from Chlorella biomass by hydrothermal liquefaction (HTL). The HTL model utilized data from a continuous 1-L reactor including catalytic hydrothermal gasification of the aqueous phase, and catalytic hydrotreatment of the HTL oil. A biophysical algae growth model coupled with weather and pond simulations predicted biomass productivity from experimental growth parameters, allowing site-by-site and temporal prediction of biomass production. The 5 BGY scale required geographically and climatically distributed sites. Even though screening down to 5 BGY significantly reduced spatial and temporal variability, site-to-site, season-to-season, and interannual variations in productivity affected economic and environmental performance. Performance metrics based on annual average or peak productivity were inadequate; temporally and spatially explicit computations allowed more rigorous analysis of these dynamic systems. For example, 3-season operation with a winter shutdown was favored to avoid high greenhouse gas emissions, but economic performance was harmed by underutilized equipment during slow-growth periods. Thus, analysis of algal biofuel pathways must combine spatiotemporal resource assessment, economic analysis, and environmental analysis integrated over many sites when assessing national scale performance.
UR - http://www.scopus.com/inward/record.url?scp=84901045149&partnerID=8YFLogxK
U2 - 10.1021/es4055719
DO - 10.1021/es4055719
M3 - Article
C2 - 24749989
AN - SCOPUS:84901045149
SN - 0013-936X
VL - 48
SP - 6035
EP - 6042
JO - Environmental Science and Technology
JF - Environmental Science and Technology
IS - 10
ER -