Practical Challenges in the Development of Photoelectrochemical Solar Fuels Production

Nathan Neale, Todd Deutsch, David Ginley, Mark Spitler, Miguel Modestino, Chengxiang Xiang, James Durrant, Daniel Esposito, Sophia Haussener, Stephen Maldonado, Ian Sharp, Bruce Parkinson, Frances Houle, Thomas Hannappel, Daniel Nocera, Paul McIntyre

Research output: Contribution to journalArticlepeer-review

58 Scopus Citations

Abstract

This article addresses the challenges presented by photoelectrochemical solar fuels technology in a discussion that begins with a functioning device and proceeds to the more fundamental science of its component parts. In this flow of discussion issues are addressed that frame the discussion for the next, increasingly more fundamental topic. The analysis begins with a discussion of the need for an analytical facility for confirmation of reported efficiencies of solar fuels device prototypes and then progressively narrows its scope to prototype design, the discovery of novel materials and the design of durable interfacial structures for fuels evolution. Molecular hydrogen will be considered first as the target fuel since many of the challenges with hydrogen production are general and applicable to the more complex CO2 reduction, which will be treated as a supplementary subject.

Original languageAmerican English
Pages (from-to)985-995
Number of pages11
JournalSustainable Energy and Fuels
Volume4
Issue number3
DOIs
StatePublished - Mar 2020

Bibliographical note

Publisher Copyright:
This journal is © The Royal Society of Chemistry.

NREL Publication Number

  • NREL/JA-5900-75059

Keywords

  • molecular hydrogen
  • photoelectrochemical
  • solar fuels
  • solar-photochemistry

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