Two Birds with One Stone: Tailoring Singlet Fission for Both Triplet Yield and Exciton Diffusion Length

Tong Zhu; Yan Wan; Zhi Guo; Justin Johnson; Libai Huang

doi:10.1002/adma.201600968

Two Birds with One Stone: Tailoring Singlet Fission for Both Triplet Yield and Exciton Diffusion Length

Tong Zhu, Yan Wan, Zhi Guo, Justin Johnson, Libai Huang

Chemistry and Nanoscience

Purdue University

Research output: Contribution to journal › Article › peer-review

71 Scopus Citations

Abstract

By direct imaging of singlet and triplet populations with ultrafast microscopy, it is shown that the triplet diffusion length and singlet fission yield can be simultaneously optimized for tetracene and its derivatives, making them ideal structures for application in bilayer solar cells.

Original language	American English
Pages (from-to)	7539-7547
Number of pages	9
Journal	Advanced Materials
Volume	28
Issue number	34
DOIs	https://doi.org/10.1002/adma.201600968 https://doi.org/10.1002/adma.201600968
State	Published - 2016

NREL Publication Number

NREL/JA-5900-65520

Keywords

exciton transport
Frenkel excitons
pump–probe microscopy
triplet fusion
ultrafast spectroscopy

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title = "Two Birds with One Stone: Tailoring Singlet Fission for Both Triplet Yield and Exciton Diffusion Length",

abstract = "By direct imaging of singlet and triplet populations with ultrafast microscopy, it is shown that the triplet diffusion length and singlet fission yield can be simultaneously optimized for tetracene and its derivatives, making them ideal structures for application in bilayer solar cells.",

keywords = "exciton transport, Frenkel excitons, pump–probe microscopy, triplet fusion, ultrafast spectroscopy",

author = "Tong Zhu and Yan Wan and Zhi Guo and Justin Johnson and Libai Huang",

year = "2016",

doi = "10.1002/adma.201600968",

language = "American English",

volume = "28",

pages = "7539--7547",

journal = "Advanced Materials",

issn = "0935-9648",

publisher = "Wiley-Blackwell",

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TY - JOUR

T1 - Two Birds with One Stone: Tailoring Singlet Fission for Both Triplet Yield and Exciton Diffusion Length

AU - Zhu, Tong

AU - Wan, Yan

AU - Guo, Zhi

AU - Johnson, Justin

AU - Huang, Libai

PY - 2016

Y1 - 2016

N2 - By direct imaging of singlet and triplet populations with ultrafast microscopy, it is shown that the triplet diffusion length and singlet fission yield can be simultaneously optimized for tetracene and its derivatives, making them ideal structures for application in bilayer solar cells.

AB - By direct imaging of singlet and triplet populations with ultrafast microscopy, it is shown that the triplet diffusion length and singlet fission yield can be simultaneously optimized for tetracene and its derivatives, making them ideal structures for application in bilayer solar cells.

KW - exciton transport

KW - Frenkel excitons

KW - pump–probe microscopy

KW - triplet fusion

KW - ultrafast spectroscopy

UR - http://www.scopus.com/inward/record.url?scp=84985963060&partnerID=8YFLogxK

U2 - 10.1002/adma.201600968

DO - 10.1002/adma.201600968

M3 - Article

C2 - 27348847

AN - SCOPUS:84985963060

SN - 0935-9648

VL - 28

SP - 7539

EP - 7547

JO - Advanced Materials

JF - Advanced Materials

IS - 34

ER -

Two Birds with One Stone: Tailoring Singlet Fission for Both Triplet Yield and Exciton Diffusion Length

Abstract

NREL Publication Number

Keywords

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