Ultrarapid Crystallization of Low-Dimensional Perovskite with Excellent Stability for Future High-Throughput Fabrication

Hongru Ma; Min Chen; Shi Wang; Qingshun Dong; Xiaopeng Zheng; Brian Wieliczka; Joseph Luther; Xuehui Liu; Yi Zhang; Jingya Guo; Mohammad Nazeeruddin; Yantao Shi

doi:10.1016/j.jpowsour.2022.232475

Ultrarapid Crystallization of Low-Dimensional Perovskite with Excellent Stability for Future High-Throughput Fabrication

Hongru Ma, Min Chen, Shi Wang, Qingshun Dong, Xiaopeng Zheng, Brian Wieliczka, Joseph Luther, Xuehui Liu, Yi Zhang, Jingya Guo, Mohammad Nazeeruddin, Yantao Shi

Chemistry and Nanoscience

Research output: Contribution to journal › Article › peer-review

3 Scopus Citations

Abstract

Perovskite solar cells (PSCs) as an emerging photovoltaic technique have achieved exceptional power conversion efficiency (PCE) up to 25.7% after fast development over the past decade. But currently some critical issues are still not well addressed in terms of realizing large-scale fabrication, for example, fast fabrication of high-quality perovskite film with good stability. Here, we demonstrate the use of stable and fast-crystallizing low-dimensional (LD) perovskite thin films as the light absorber with only a 10 s annealing time at 250 °C, delivering a PCE of 18.16%. The crystallization and photoelectric properties of LD perovskite are well illustrated. The reduction in the annealing time will dramatically increase the productivity of PSCs. The PSCs based on rapidly annealed LD perovskite thin films exhibit excellent stability, with only 12% loss of PCE after 1000 h storage at 85 °C and 40–70% relative humidity.

Original language	American English
Article number	232475
Number of pages	7
Journal	Journal of Power Sources
Volume	556
DOIs	https://doi.org/10.1016/j.jpowsour.2022.232475 https://doi.org/10.1016/j.jpowsour.2022.232475
State	Published - 1 Feb 2023

Bibliographical note

Publisher Copyright:
© 2022 Elsevier B.V.

NREL Publication Number

NREL/JA-5900-84947

Keywords

Fast crystallizing
Low-dimensional perovskite
Perovskite solar cells
Stability

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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Ma, H., Chen, M., Wang, S., Dong, Q., Zheng, X., Wieliczka, B., Luther, J., Liu, X., Zhang, Y., Guo, J., Nazeeruddin, M., & Shi, Y. (2023). Ultrarapid Crystallization of Low-Dimensional Perovskite with Excellent Stability for Future High-Throughput Fabrication. Journal of Power Sources, 556, Article 232475. https://doi.org/10.1016/j.jpowsour.2022.232475, https://doi.org/10.1016/j.jpowsour.2022.232475

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title = "Ultrarapid Crystallization of Low-Dimensional Perovskite with Excellent Stability for Future High-Throughput Fabrication",

abstract = "Perovskite solar cells (PSCs) as an emerging photovoltaic technique have achieved exceptional power conversion efficiency (PCE) up to 25.7% after fast development over the past decade. But currently some critical issues are still not well addressed in terms of realizing large-scale fabrication, for example, fast fabrication of high-quality perovskite film with good stability. Here, we demonstrate the use of stable and fast-crystallizing low-dimensional (LD) perovskite thin films as the light absorber with only a 10 s annealing time at 250 °C, delivering a PCE of 18.16%. The crystallization and photoelectric properties of LD perovskite are well illustrated. The reduction in the annealing time will dramatically increase the productivity of PSCs. The PSCs based on rapidly annealed LD perovskite thin films exhibit excellent stability, with only 12% loss of PCE after 1000 h storage at 85 °C and 40–70% relative humidity.",

keywords = "Fast crystallizing, Low-dimensional perovskite, Perovskite solar cells, Stability",

author = "Hongru Ma and Min Chen and Shi Wang and Qingshun Dong and Xiaopeng Zheng and Brian Wieliczka and Joseph Luther and Xuehui Liu and Yi Zhang and Jingya Guo and Mohammad Nazeeruddin and Yantao Shi",

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Ma, H, Chen, M, Wang, S, Dong, Q, Zheng, X, Wieliczka, B, Luther, J, Liu, X, Zhang, Y, Guo, J, Nazeeruddin, M & Shi, Y 2023, 'Ultrarapid Crystallization of Low-Dimensional Perovskite with Excellent Stability for Future High-Throughput Fabrication', Journal of Power Sources, vol. 556, 232475. https://doi.org/10.1016/j.jpowsour.2022.232475, https://doi.org/10.1016/j.jpowsour.2022.232475

TY - JOUR

T1 - Ultrarapid Crystallization of Low-Dimensional Perovskite with Excellent Stability for Future High-Throughput Fabrication

AU - Ma, Hongru

AU - Chen, Min

AU - Wang, Shi

AU - Dong, Qingshun

AU - Zheng, Xiaopeng

AU - Wieliczka, Brian

AU - Luther, Joseph

AU - Liu, Xuehui

AU - Zhang, Yi

AU - Guo, Jingya

AU - Nazeeruddin, Mohammad

AU - Shi, Yantao

PY - 2023/2/1

Y1 - 2023/2/1

N2 - Perovskite solar cells (PSCs) as an emerging photovoltaic technique have achieved exceptional power conversion efficiency (PCE) up to 25.7% after fast development over the past decade. But currently some critical issues are still not well addressed in terms of realizing large-scale fabrication, for example, fast fabrication of high-quality perovskite film with good stability. Here, we demonstrate the use of stable and fast-crystallizing low-dimensional (LD) perovskite thin films as the light absorber with only a 10 s annealing time at 250 °C, delivering a PCE of 18.16%. The crystallization and photoelectric properties of LD perovskite are well illustrated. The reduction in the annealing time will dramatically increase the productivity of PSCs. The PSCs based on rapidly annealed LD perovskite thin films exhibit excellent stability, with only 12% loss of PCE after 1000 h storage at 85 °C and 40–70% relative humidity.

AB - Perovskite solar cells (PSCs) as an emerging photovoltaic technique have achieved exceptional power conversion efficiency (PCE) up to 25.7% after fast development over the past decade. But currently some critical issues are still not well addressed in terms of realizing large-scale fabrication, for example, fast fabrication of high-quality perovskite film with good stability. Here, we demonstrate the use of stable and fast-crystallizing low-dimensional (LD) perovskite thin films as the light absorber with only a 10 s annealing time at 250 °C, delivering a PCE of 18.16%. The crystallization and photoelectric properties of LD perovskite are well illustrated. The reduction in the annealing time will dramatically increase the productivity of PSCs. The PSCs based on rapidly annealed LD perovskite thin films exhibit excellent stability, with only 12% loss of PCE after 1000 h storage at 85 °C and 40–70% relative humidity.

KW - Fast crystallizing

KW - Low-dimensional perovskite

KW - Perovskite solar cells

KW - Stability

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DO - 10.1016/j.jpowsour.2022.232475

M3 - Article

AN - SCOPUS:85144019507

SN - 0378-7753

VL - 556

JO - Journal of Power Sources

JF - Journal of Power Sources

M1 - 232475

ER -

Ultrarapid Crystallization of Low-Dimensional Perovskite with Excellent Stability for Future High-Throughput Fabrication

Abstract

Bibliographical note

NREL Publication Number

Keywords

UN SDGs

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